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Lattice matching and microstructuring of Gd3+, Lu3+ co-doped KY(WO4)2:Tm3+ channel waveguide lasers

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Lattice matching and microstructuring of Gd

3+

, Lu

3+

co-doped KY(WO

4

)

2

:Tm

3+

Channel Waveguide Lasers

K. van Dalfsen, S. Aravazhi, D. Geskus, K. Wörhoff, and M. Pollnau

Integrated Optical MicroSystems Group, MESA+ Institute for Nanotechnology, University of Twente,

PO Box 217, 7500 AE, Enschede, The Netherlands Author e-mail address: k.vandalfsen@utwente.nl

Abstract: Lattice-matched KY(WO4)2:Gd3+,Lu3+,Tm3+ layers with a thickness of 6 µm have been

grown onto pure KY(WO4)2 substrates. Channel waveguides of 7.5 µm to 12.5 µm width have

been microstructured to a depth of 1.5 µm using Ar+ beam milling. Laser experiments with butt-coupled mirrors demonstrate laser oscillation near 1844 nm while pumping at 792 nm.

Planar waveguide lasers in KYW:Tm have been demonstrated in an open cavity configuration [1]. In this paper we report on the fabrication and preliminary performance of channel waveguide lasers in KYW:Tm.

KYW thin layers co-doped with Gd3+, Lu3+, and a Tm3+ concentration of 1.5 at.% were grown by liquid-phase epitaxy from a K2W2O7 solvent onto undoped KYW substrates. The compressive and tensile strains are balanced

out by combining a doping concentration of 19.6 at.% Gd3+ and 18.9 at.% Lu3+, minimizing the lattice stress [2]. Besides, a refractive index contrast of 6×10-3

between the grown layer and the substrate was obtained by replacing Y3+ with optically inert Gd3+ and Lu3+ ions, both of which exhibit higher refractive indices [3,4]. The obtained refractive index contrast ensures strong confinement along the b-crystallographic axis of the pump and laser modes at 802 nm and 1844 nm, respectively, while fabrication of ridge-type waveguides is facilitated by the shallow etch-depth requirements due to the small layer thickness. Single-mode laser operation in ridge-type waveguides is expected for a layer thickness of 6 µm, channel widths of 7.5–12.5 µm, and 4.5 µm remaining slab thickness.

A grown co-doped layer was lapped and polished down to the required thickness of 6 µm, after which a layer of photoresist (Fujifilm OiR 908/35) was deposited and patterned. Ar+ beam milling of the rotating sample with an energy of 350 eV was used to imprint the channel pattern along the Ng optical axis into the optically active layer at a

rate of 3 nm/min [5]. A scanning electron microscope (SEM) image of the resulting waveguides is shown in Fig. 1a. The patterned layer is overgrown with a pure KYW layer to reduce the optical loss and ensure good overlap between pump and laser modes.

Laser experiments with butt-coupled mirrors have been conducted on the KYW:Tm channel waveguide samples, showing laser operation at 1844 nm while pumping at 792 nm in Np polarization, see Figs. 1b and 1c.

Funding was provided by the IOP Photonic Devices Program of the Dutch funding agencies Senter-Novem and STW under project PD-55 “On-chip Integrated NH3 Human Gas Sensor”.

Fig. 1. (a) SEM micrograph of a ridge-type channel waveguide microstructured by Ar+ milling, (b) emission spectrum and

(c) relaxation oscillations of a KYW:Tm channel waveguide laser

[1] S. Rivier, X. Mateos, V. Petrov, U. Griebner, Y. E. Romanyuk, C. N. Borna, F. Gardillou, and M. Pollnau, Opt. Express 15, 5885 (2007). [2] F. Gardillou, Y. E. Romanyuk, C. N. Borca, R. P. Salathé, and M. Pollnau, Opt. Lett. 32, 488 (2007).

[3] M. C. Pujol X. Mateos, A. Aznar, X. Solans, S. Surinach, J. Massons, F. Diaz, and M. Aguilo, J. Appl. Cryst. 39, 2, 230-236 (2006). [4] M. C. Pujol, X. Mateos, R. Sole, J. Massons, Jna Gavalda, F. Diaz, and M. Aguilo, Materials Science Forum Vols., 378-381, 710-717

(2001).

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