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Angular dependence of Josephson currents in unconventional superconducting junctions

T. Yokoyama,1Y. Sawa,1Y. Tanaka,1and A. A. Golubov2

1Department of Applied Physics, Nagoya University, Nagoya, 464-8603, Japan and CREST, Japan Science and Technology Corporation (JST) Nagoya, 464-8603, Japan 2Faculty of Science and Technology, University of Twente, 7500 AE, Enschede, The Netherlands

共Received 26 September 2006; published 3 January 2007兲

Josephson effect in junctions between unconventional superconductors is studied theoretically within the model describing the effects of interface roughness. The particularly important issue of applicability of the frequently used Sigrist-Rice共SR兲 formula for Josephson current in d-wave superconductor/insulator/d-wave superconductor junctions is addressed. We show that although the SR formula is not applicable in the ballistic case, it works well for rough interfaces when the diffusive normal metal regions exist between the d-wave superconductor and the insulator. It is shown that the SR approach only takes into account the component of the d-wave pair potential symmetric with respect to an inversion around the plane perpendicular to the inter-face. Similar formula can be derived for general unconventional superconductors with arbitrary angular mo-mentum l.

DOI:10.1103/PhysRevB.75.020502 PACS number共s兲: 74.20.Rp, 74.50.⫹r, 74.70.Kn

A number of phase-sensitive experiments have convinc-ingly demonstrated the realization of d-wave pairing state in high-TC cuprates.1–4 Because of such unconventional sym-metry, the study of Josephson effect in high-TC supercon-ducting共HTS兲 junctions attracted a lot of interest. A while ago, a simple formula for the Josephson current of d-wave superconductor/insulator/d-wave superconductor 共DID兲 junctions was proposed by Sigrist and Rice共SR兲.5According

to the SR formula, the Josephson current is proportional to cos 2␣cos 2␤, where the␣共␤兲 denotes the angle between the normal to the interface and the crystal axis of the left共right兲

d-wave superconductor.5

Although the SR formula can explain experiments with the so-called␲ junctions,1,2 this formula does not take into

account the effect of midgap Andreev resonant states 共MARS兲 formed at junction interfaces.6,7Actually, as shown

in Ref. 8, SR formula does not work in ballistic d-wave junctions for ␣⫽0 and ␤⫽0 where MARS influence se-verely the charge transport at low temperatures. It was shown both theoretically9,10 and experimentally11,12 that MARS

in-duce a nonmonotonic temperature dependence of the maxi-mum Josephson current in DID junctions. On the other hand, SR formula has been extensively used to analyze experi-ments with various types of HTS Josephson junctions.13–15

Experiments with HTS junctions are of high importance for basic understanding of high-Tc superconductivity since they may provide information on possible subdominant admix-tures to the d-wave symmetry.16–18Therefore it is of

funda-mental interest to understand the physical mechanisms that determine the angular dependence of Josephson current in HTS junctions. For this reason, the determination of the con-ditions of applicability of the SR formula is an important issue which is addressed in the present paper.

In the following, we study the Josephson current in

D / DN/ I / DN/ D junctions, where DN denotes diffusive

nor-mal metal and could be formed between the insulator and

d-wave superconductors. The calculations are based on the

quasiclassical Green’s function method applicable to uncon-ventional superconductor junctions.19,20 We find that the

re-sulting Josephson current in D / DN/ I / DN/ D junctions is well fitted by the SR formula. Near the transition tempera-ture, it is proven analytically that Josephson current follows the SR formula. We also confirm that this formula does not hold in the ballistic junctions. It is clarified that in the SR formula, the component of the pair potential that is antisym-metric by the inversion operation around the plane perpen-dicular to the interface is neglected. We also study p-wave superconductor/diffusive normal metal/insulator/diffusive normal metal/p-wave superconductor 共P/DN/I/DN/ P兲 junctions. The resulting Josephson current is also well fitted by cos␣cos␤, where ␣ 共␤兲 denotes the angle between the crystal axis of left 共right兲 p-wave superconductor and the normal to the interface. This is a corresponding version of the SR formula in the p-wave superconductor junctions. Fur-thermore, it is possible to extend the theory for an unconven-tional superconductor 共US兲 with arbitrary angular momen-tum l. For US/DN/I/DN/US junctions, the expected Josephson current is proportional to cos lcos l␤. The ob-tained results may serve as a guide for the analysis of the experiments in unconventional superconductor junctions.

Before we proceed with a formal discussion, let us provide qualitative arguments on the physical meaning of the SR formula and explain why it holds in the diffusive junctions. First, we consider d-wave supercon-ductor junctions. The pair potentials of left and right

d-wave superconductors are, respectively, expressed byL =⌬关fSL共␾兲+ fASL共␾兲兴exp共−i⌿兲, and ⌬R=⌬关fSR共␾兲+ fASR共␾兲兴, with fSL共␾兲=cos 2␾cos 2␣, fASL共␾兲=sin 2␾sin 2␣, fSR共␾兲 = cos 2␾cos 2␤, fASR共␾兲=sin 2␾sin 2␤, where ␾ is the in-jection angle measured from the interface normal,⌬ denotes the maximum value of the pair potential and⌿ is the phase difference across the junction. The terms proportional to cos 2␾, i.e., fSL共␾兲 and fSR共␾兲, correspond to the dx2−y2-wave pair potential and the terms proportional to sin共2␾兲, i.e.,

fASL共␾兲 and fASR共␾兲, correspond to the dxy-wave pair poten-tial, respectively. Here, fSL共␾兲= fSL共−␾兲, fSR共␾兲= fSR共−␾兲,

fASL共␾兲=−fASL共−␾兲, and fASR共␾兲=−fASR共−␾兲 are satisfied. In the actual calculation of Josephson current in

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D / DN/ I / DN/ D junctions, we have to take an average over

the various ␾. Due to the impurity scattering in DN, the average is taken for the left and right D/DN interface inde-pendently. Then we can drop fASL共␾兲 and fASR共␾兲 and arrive at the SR formula, where only the terms fSL共␾兲 and fSR共␾兲 remain which do not change sign by exchanging␾ for −␾. This fact is in accordance with the recent result that the prox-imity effect is absent in the case of dxy-wave pair potential.19 Consequently, the resulting Josephson current is proportional to cos 2␣cos 2␤.

Similar arguments apply to p-wave junctions. In this case, fSL共␾兲=cos␾cos␣, fASL共␾兲=sin␾sin␣, fSR共␾兲 = cos␾cos␤, and fASR共␾兲=sin␾sin␤ are satisfied. The terms proportional to cos␾, i.e., fSL共␾兲 and fSR共␾兲, corre-spond to the px-wave pair potential and the terms propor-tional to sin␾, i.e., fASL共␾兲 and fASR共␾兲, correspond to the

py-wave pair potential. In the actual calculation for

P / DN/ I / DN/ P junctions, functions fASL共␾兲 and fASR共␾兲 vanish after averaging over angle␾. This is consistent with our previous results that the pair potential with py-wave sym-metry does not contribute to the proximity effect.21,22

Next we formulate the junction model and basic equations starting from the d-wave case. We consider ballistic DID and

D / DN/ I / DN/ D junctions. The DN has a resistance Rdand a length L much larger than the mean free path. The DN/D interfaces located at x = ± L have the resistance Rb

, while the DN/I interface at x = 0 has the resistance Rb. We model infi-nitely narrow insulating barriers by the delta function U共x兲 = H

共x+L兲+H共x兲+H

共x−L兲. The resulting transparen-cies of the junctions Tm and Tm

are given by Tm = 4 cos2/共4 cos2+ Z2兲 and T

m

= 4 cos2/共4 cos2+ Z

2兲, where Z = 2H /vF and Z

= 2H

/vF are dimensionless con-stants共we take ប=kB= 1 in this paper兲 and vF is Fermi ve-locity. Below we assume Z1. The schematic illustration of the models is shown in Fig. 1. Here, ␣ and ␤ denote the angles between the normal to the interface and the crystal axis of the left and right d-wave共or p-wave兲

superconduct-ors, respectively. The lobe direction of the pair potential and the direction of the crystal axis are chosen to be the same. The pair potential along the quasiparticle trajectory with the injection angle␾ is given by ⌬L=⌬ cos关2共␾−␣兲兴exp共−i⌿兲 and⌬R=⌬ cos关2共␾−␤兲兴 for the left and the right supercon-ductor, respectively. For ballistic junctions, we use a similar model without DN and calculate the Josephson current fol-lowing Ref.9.

We parametrize the quasiclassical Green functions G and

F with a function:23,24 G=

␻ ␻2+ ␻⌽−␻* , F=

⌽␻ ␻2+ ␻⌽−␻* , 共1兲

where␻is the Matsubara frequency. Then the Usadel equa-tion reads25 ␰2␲TCG ⳵ ⳵x

G␻ 2 ⳵ ⳵x⌽␻

−⌽␻= 0 共2兲

with the coherence length ␰=

D / 2TC, the diffusion con-stant D and the transition temperature TC. We solve the Us-adel equation with the boundary conditions in Ref.20 at x = ± L and those in Ref.26at x = 0.

The Josephson current is given by

eIRTC = i RTL 2RdTC

G2 ␻2

⌽␻ ⳵ ⳵x⌽−␻ * −␻ * ⳵ ⳵x⌽␻

, 共3兲

where T is temperature and R⬅2Rd+ Rb+ 2Rb

is the normal state resistance of the junction. In the following we focus on the ICR value where ICdenotes the magnitude of the maxi-mum Josephson current. We fix parameters as Z

= 0, Rd/ Rb = 0.01, Rd/ Rb

= 10, and ETh/⌬0= 1 for D / DN/ I / DN/ D junc-tions and Z = 10 for DID juncjunc-tions.0denotes the value of⌬ at zero temperature. The choice of the small magnitude of Z

and Rb

and large Thouless energy is justified by the fact that thin DN could be naturally formed due to the degradation of superconductivity near the interface.

The ␣ dependence of ICR for d-wave superconductor junctions is plotted in Fig.2. In Figs. 2共a兲and2共b兲, ICR of ballistic junctions is plotted for low 共T/TC= 0.2兲 and high temperature 共T/TC= 0.9兲, respectively. With the increase of the magnitude of␤, the dependence of ICR on ␣transforms from cos 2␣ to sin 2␣. These␣ dependences cannot be ex-pressed by the SR formula, where ICR is proportional to cos 2␣ for fixed ␤. On the other hand in D / DN/ I / DN/ D junctions, ICR has a simple form, cos 2␣, independent of␤at low and high temperatures as shown in Figs.2共c兲and2共d兲, respectively. The magnitudes of ICR in D / DN/ I / DN/ D junctions are at least two orders smaller than those in DID junctions. By taking account of the ␤ dependence, ICR is almost proportional to cos 2␣cos 2␤. It should be remarked that this fitting is possible for small magnitude of Z

and

Rb

/ Rdwhere the MARS formed at the D/DN interface do not influence seriously the charge transport.

The corresponding results of ICR for p-wave supercon-ductor junctions are plotted in Fig. 3. For P / DN/ I / DN/ P junctions, ICR can be fitted by cos␣cos␤. Similar to the case of d-wave junctions, this fitting is possible for small

FIG. 1. 共Color online兲 Schematic illustration of the models of 共a兲 D/DN/I/DN/D and 共b兲 P/DN/I/DN/ P junctions.

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magnitude of Z

and Rb

/ Rd. For ballistic junctions, as shown in Figs.3共a兲and3共b兲, this fitting does not work any more.

In the following, we will present analytical result demon-strating why the SR formula does not work in ballistic junc-tions and works in the diffusive juncjunc-tions. Although we focus on d-wave junctions, similar discussion is possible for

p-wave junctions. Near TC共⌬␻兲, we can get the formula for the ballistic DID junctions9

eIRTC =⌬ 2sin 8TTC F0,

F0=具cos22␾典cos 2␣cos 2␤+具sin22␾典sin 2␣sin 2␤. 共4兲 Here, the average over the various angles of injected par-ticles at the interfaces is defined as

具B共␾兲典 =

−␲/2 ␲/2 dT共␾兲cos␾B共␾兲

−␲/2 ␲/2 dT共␾兲cos␾ 共5兲

with T共兲=Tm. It is easy to check that 具cos22␾典 and 具sin22典 are of the same order for all Z. Therefore, SR for-mula cannot be applicable to nonzero values of ␣ and ␤. Also we can roughly estimate the Josephson current

eIR

TC ⬵ ⌬2

16TTC

cos共2␣− 2␤兲sin ⌿ 共6兲 which is consistent with the result in Fig.2共b兲. In the case of

PIP junctions, we can obtain the corresponding equation by

replacing 2␣, 2␤, and 2␾ with ␣, ␤, and ␾ in the above equations.

Next we consider the D / DN/ I / DN/ D junctions. Near TC, we can linearize the Usadel equation as follows:

␰2⳵ 2 ⳵x2⌽j␻− ␻ ␲TCj␻= 0, 共7兲

where j共=1,2兲 denotes the left or right DN. Similarly the boundary conditions at x = −L, x = 0, and x = L are reduced to

⳵ ⳵x⌽1␻

x=−L= − Rd Rb

L 共− ⌽1␻+ I0cos 2␣e−i⌿兲

x=−L , 共8兲

⳵⌽1␻ ⳵x

x=0 = ⳵⌽2␻ ⳵x

x=0= Rd共⌽2␻−⌽1␻兲 RbL

x=0 , 共9兲 ⳵⌽2␻ ⳵x

x=L= Rd Rb

L 共− ⌽2␻+ I0cos 2␤兲

x=L 共10兲 with I0=⌬具cos 2␾典.

Solving the above equations, we find the expression for the Josephson current of the form

eIRTC =Rrr

2 Rd T TC

L具cos 2␾典2⌬2cos 2␣cos 2␤sin⌿

␻2F 1F2 , F1=␥L sinhL + r

cosh␥L, F2=关共2rr

+␥2L2兲sinh␥L +共2r + r

兲␥L coshL兴 共11兲 with r =Rd Rb, r

= Rd Rb⬘, and ␥=

2␻

D. Thus the SR formula is proven to be valid near TC. In the case of P/DN/I/DN/P junctions, cos 2␾, cos 2␣, and cos 2␤ have to be replaced with cos␾, cos␣, and cos␤, respectively, to obtain the cor-responding formula. This result is consistent with the previ-ous study of DID junctions with rough interface,27where the

SR formula is applicable as well.

In order to understand the above results qualitatively, let us discuss the symmetry of the pair potential by the inversion operation around the plane perpendicular to the interface. As shown in Fig. 4, dx2−y2 wave and px wave are symmetric while dxywave and pywave are antisymmetric by this op-eration. Only the symmetric pair wave function is taken into

FIG. 2.共Color online兲 Maximum Josephson current for d-wave junctions.共a兲 and 共b兲 DID junctions. 共c兲 and 共d兲 D/DN/I/DN/D junctions. Solid lines in共c兲, 共d兲 are proportional to cos 2␣ cos 2␤.

FIG. 3.共Color online兲 Maximum Josephson current for p-wave junctions.共a兲 and 共b兲 PIP junctions. 共c兲 and 共d兲 P/DN/I/DN/ P junctions with solid lines that are proportional to cos␣ cos ␤.

ANGULAR DEPENDENCE OF JOSEPHSON CURRENTS IN… PHYSICAL REVIEW B 75, 020502共R兲 共2007兲 RAPID COMMUNICATIONS

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account in the SR formula. Applying this idea to an arbitrary unconventional superconductor with angular momentum l, one can argue that the Josephson current is proportional to cos lcos l␤. It is straightforward to get this result just by

replacing cos 2␾, cos 2␣, and cos 2␤ with cos l, cos l␣, and cos l␤ in Eq.共11兲, respectively.

In summary, we have studied the validity and the physical meaning of the Sigrist-Rice formula in d-wave supercon-ductor junctions. According to the SR formula, the amplitude of the maximum Josephson current is proportional to cos 2␣cos 2␤. Although this formula is not applicable to the ballistic junctions, it works well for D/DN/I/DN/D junctions where the DN regions are located between the d-wave super-conductor and the insulator. We have also shown that in

P/DN/I/DN/P junctions, the Josephson current is

propor-tional to cos␣cos␤. The obtained results may help to obtain information about pairing symmetry in experiments with un-conventional superconducting junctions.

T. Y. acknowledges support by the JSPS. This work is supported by Grant-in-Aid for Scientific Research on Priority Area “Novel Quantum Phenomena Specific to Anisotropic Superconductivity”共Grant No. 17071007兲 from the Ministry of Education, Culture, Sports, Science and Technology of Japan.

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The␾ dependences are given by cos 2␾, cos ␾, sin 2␾, and sin ␾.

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